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Therefore, this study was aimed to produce high-performance concrete by incorporating a high volume of basaltic volcanic ash along with metakaolin (MK), micro-silica (MS), and nano-silica (NS). An investigation was performed in regard to the mechanical and durability properties, autogenous and drying shrinkage, and microstructural and pore-structure properties. A control mix, binary mixes, and ternary mixes were examined. The binary mixes contained fine (VA) and ultra-fine (VAF) volcanic ashes, and the ternary mixes contained combinations of VA with MK, MS, and NS. Test results show that ternary mixes with 30% and 40% cement substitution demonstrated better strength development and higher resistance to chloride penetration and water absorption. All binary and ternary mixes displayed lower autogenous shrinkage, as well as lower or comparable drying shrinkage than the control mix. Moreover, the combination of VA with MK, MS, and NS up to 40% resulted in micro and pore structure refinement by forming high-density gels. 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