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Recent Advances of VO2 in Sensors and Actuators
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Vanadium dioxide (VO2) stands out for its versatility in numerous applications, thanks to its unique reversible insulator-to-metal phase transition. This transition can be initiated by various stimuli, leading to significant alterations in the material’s characteristics, including its resistivity and optical properties. As the interest in the material is growing year by year, the purpose of this review is to explore the trends and current state of progress on some of the applications proposed for VO2 in the field of sensors and actuators using literature review methods. Some key applications identified are resistive sensors such as strain, temperature, light, gas concentration, and thermal fluid flow sensors for microfluidics and mechanical microactuators. Several critical challenges have been recognized in the field, including the expanded investigation of VO2-based applications across multiple domains, exploring various methods to enhance device performance such as modifying the phase transition temperature, advancing the fabrication techniques for VO2 structures, and developing innovative modelling approaches. Current research in the field shows a variety of different sensors, actuators, and material combinations, leading to different sensor and actuator performance input ranges and output sensitivities.
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<div class="JournalArticle Publication short-list"> <div class="authors"> <span class="author-name" mtid="10065089"> <a href="/gui2/?type=authors&mode=browse&sel=10065089" target="_blank">Darwish, Mahmoud ✉</a> </span> <span class="author-type"> </span> ; <span class="author-name" > Zhabura, Yana </span> <span class="author-type"> </span> ; <span class="author-name" mtid="10041061"> <a href="/gui2/?type=authors&mode=browse&sel=10041061" target="_blank">Pohl, László ✉</a> </span> <span class="author-type"> </span> </div ><div class="title"><a href="/gui2/?mode=browse¶ms=publication;34761133" mtid="34761133" target="_blank">Recent Advances of VO2 in Sensors and Actuators</a></div> <div class="pub-info"> <span class="journal-title">NANOMATERIALS</span> <span class="journal-volume">14</span> : <span class="journal-issue">7</span> <span class="page"> pp. 1-22. Paper: 582 , 22 p. </span> <span class="year">(2024)</span> </div> <div class="pub-end"><div class="identifier-list"> <span class="identifiers"> <span class="id identifier oa_none" title="none"> <a style="color:black" title="10.3390/nano14070582" target="_blank" href="https://doi.org/10.3390/nano14070582"> DOI </a> </span> <span class="id identifier oa_none" title="none"> <a style="color:black" title="https://www.mdpi.com/2079-4991/14/7/582" target="_blank" href="https://www.mdpi.com/2079-4991/14/7/582"> Egyéb URL </a> </span> </span> </div> <div class="short-pub-prop-list"> <span class="short-pub-mtid"> Közlemény:34761133 </span> <span class="status-holder"><span class="status-data status-APPROVED"> Nyilvános </span></span> <span class="pub-core">Forrás </span> <span class="pub-type">Folyóiratcikk (Szakcikk ) </span> <!-- && !record.category.scientific --> <span class="pub-category">Tudományos</span> </div> </div> </div><div class="JournalArticle Publication long-list"> <div class="authors"> <img title="Forrásközlemény" style="float: left" src="/frontend/resources/grid/publication-core-icon.png"> <div class="autype autype0"> <span class="author-name" mtid="10065089"><a href="/gui2/?type=authors&mode=browse&sel=10065089" target="_blank">Darwish Mahmoud ✉ (<span class="authorship-author-name">Darwish Mahmoud Ibrahim Azmi</span> <span class="authorAux-mtmt"> villamosmérnöki tudományok</span>) </a> </span> ; <span class="author-name" >Zhabura Yana </span> ; <span class="author-name" mtid="10041061"><a href="/gui2/?type=authors&mode=browse&sel=10041061" target="_blank">Pohl László ✉ (<span class="authorship-author-name">Pohl László</span> <span class="authorAux-mtmt"> elektronika</span>) </a> </span> </div> </div> <div class="title"><a href="/gui2/?mode=browse¶ms=publication;34761133" target="_blank">Recent Advances of VO2 in Sensors and Actuators</a></div> <div> <span class="journal-title">NANOMATERIALS</span> <span class="journal-issn">( <a target="_blank" href="https://portal.issn.org/resource/ISSN/2079-4991">2079-4991</a>)</span>: <span class="journal-volume">14</span> <span class="journal-issue">7</span> <span class="page"> pp 1-22 Paper 582. </span> <span class="year">(2024)</span> </div> <div class="pub-footer"> <span class="language" xmlns="http://www.w3.org/1999/html">Nyelv: Angol | </span> <span class="identifiers"> <span class="id identifier oa_none" title="none"> <a style="color:black" title="10.3390/nano14070582" target="_blank" href="https://doi.org/10.3390/nano14070582"> DOI </a> </span> <span class="id identifier oa_none" title="none"> <a style="color:black" title="https://www.mdpi.com/2079-4991/14/7/582" target="_blank" href="https://www.mdpi.com/2079-4991/14/7/582"> Egyéb URL </a> </span> </span> <div class="mtid"><span class="long-pub-mtid">Közlemény: 34761133</span> | <span class="status-data status-APPROVED"> Nyilvános </span> Forrás | <span class="type-subtype">Folyóiratcikk ( Szakcikk ) </span> | <span class="pub-category">Tudományos</span> | <span class="publication-sourceOfData">kézi felvitel</span> </div> <div class="lastModified">Utolsó módosítás: 2024.03.28. 20:52 Pohl László (elektronika) </div> </div></div>
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Romano, Eugenia
Enhanced Stability of Oral Vitamin C Delivery: A Novel Large-Scale Method for Liposomes Production and Encapsulation through Dynamic High-Pressure Microfluidization
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In recent years, nanocarriers have been widely used as an effective solution for oral administration of pharmaceuticals. However, there is still an urgent need to speed up their translation to clinical practice. Cost-effective and industrially scalable methodologies are still needed. Herein, the production of vitamin C-loaded liposomes for nutraceutical purposes has been investigated and optimized by adopting a High-Pressure Homogenizer. Initially, the impact of process parameters on particles size, distributions, and morphology was explored. The findings document that the pressure and cycle manipulation allow for control over liposome size and polydispersity, reaching a maximum encapsulation efficiency exceeding 80%. This significantly improves the storage stability of vitamin C, as demonstrated by monitoring its antioxidant activity. Furthermore, the in vitro simulation of gastrointestinal digestion shows that liposomes could protect the active substance from damage and control its release in the gastrointestinal fluid. Thus, the whole nanodelivery system can contribute to enhancing vitamin C bioavailability. In conclusion, the results indicate that this innovative approach to producing vitamin C liposomes holds promise for clinical translation and industrial scale-up. Indeed, by utilizing food-grade materials and straightforward equipment, it is possible to produce stable and functional liposomes suitable for health products.
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<div class="JournalArticle Publication short-list"> <div class="authors"> <span class="author-name" > Romano, Eugenia </span> <span class="author-type"> </span> ; <span class="author-name" > Palladino, Roberta </span> <span class="author-type"> </span> ; <span class="author-name" > Cannavale, Mariagabriella </span> <span class="author-type"> </span> ; <span class="author-name" > Lamparelli, Erwin Pavel </span> <span class="author-type"> </span> ; <span class="author-name" > Maglione, Barbara </span> <span class="author-type"> </span> </div ><div class="title"><a href="/gui2/?mode=browse¶ms=publication;34761436" mtid="34761436" target="_blank">Enhanced Stability of Oral Vitamin C Delivery: A Novel Large-Scale Method for Liposomes Production and Encapsulation through Dynamic High-Pressure Microfluidization</a></div> <div class="pub-info"> <span class="journal-title">NANOMATERIALS</span> <span class="journal-volume">14</span> : <span class="journal-issue">6</span> <span class="page"> p. 516 </span> <span class="year">(2024)</span> </div> <div class="pub-end"><div class="identifier-list"> <span class="identifiers"> <span class="id identifier oa_none" title="none"> <a style="color:black" title="10.3390/nano14060516" target="_blank" href="https://doi.org/10.3390/nano14060516"> DOI </a> </span> <span class="id identifier oa_none" title="none"> <a style="color:black" title="https://www.mdpi.com/2079-4991/14/6/516" target="_blank" href="https://www.mdpi.com/2079-4991/14/6/516"> Egyéb URL </a> </span> </span> </div> <div class="short-pub-prop-list"> <span class="short-pub-mtid"> Közlemény:34761436 </span> <span class="status-holder"><span class="status-data status-APPROVED"> Nyilvános </span></span> <span class="pub-core"> Idéző </span> <span class="pub-type">Folyóiratcikk (Szakcikk ) </span> <!-- && !record.category.scientific --> <span class="pub-category">Tudományos</span> </div> </div> </div><div class="JournalArticle Publication long-list"> <div class="authors"> <img title="Idézőközlemény" style="float: left" src="/frontend/resources/grid/publication-citation-icon.png"> <div class="autype autype0"> <span class="author-name" >Romano Eugenia </span> ; <span class="author-name" >Palladino Roberta </span> ; <span class="author-name" >Cannavale Mariagabriella </span> ; <span class="author-name" >Lamparelli Erwin Pavel </span> ; <span class="author-name" >Maglione Barbara </span> </div> </div> <div class="title"><a href="/gui2/?mode=browse¶ms=publication;34761436" target="_blank">Enhanced Stability of Oral Vitamin C Delivery: A Novel Large-Scale Method for Liposomes Production and Encapsulation through Dynamic High-Pressure Microfluidization</a></div> <div> <span class="journal-title">NANOMATERIALS</span> <span class="journal-issn">( <a target="_blank" href="https://portal.issn.org/resource/ISSN/2079-4991">2079-4991</a>)</span>: <span class="journal-volume">14</span> <span class="journal-issue">6</span> <span class="page"> p. 516. </span> <span class="year">(2024)</span> </div> <div class="pub-footer"> <span class="language" xmlns="http://www.w3.org/1999/html">Nyelv: Angol | </span> <span class="identifiers"> <span class="id identifier oa_none" title="none"> <a style="color:black" title="10.3390/nano14060516" target="_blank" href="https://doi.org/10.3390/nano14060516"> DOI </a> </span> <span class="id identifier oa_none" title="none"> <a style="color:black" title="https://www.mdpi.com/2079-4991/14/6/516" target="_blank" href="https://www.mdpi.com/2079-4991/14/6/516"> Egyéb URL </a> </span> </span> <div class="publication-citation"> <a target="_blank" href="/api/publication?cond=citations.related;eq;34761436&sort=publishedYear,desc&sort=title"> Idézett közlemények száma: 1 </a> </div> <div class="mtid"><span class="long-pub-mtid">Közlemény: 34761436</span> | <span class="status-data status-APPROVED"> Nyilvános </span> Idéző | <span class="type-subtype">Folyóiratcikk ( Szakcikk ) </span> | <span class="pub-category">Tudományos</span> | <span class="publication-sourceOfData">kézi felvitel</span> </div> <div class="lastModified">Utolsó módosítás: 2024.03.28. 12:45 Sipos Bence (Gyógyszertechnológia) </div> </div></div>
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Lei, Da-Peng
Automated Monitoring System for Suspended Photocatalytic Batch Reactions Based on Online Circulatory Spectrophotometry
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Employing an automated monitoring system (AMS) for data acquisition offers benefits, such as reducing the workload, in the kinetic study of suspended photocatalytic batch reactions. However, the current methods in this field tend to narrowly focus on the substrate and often overlook the optical characteristics of both the mixture and solid particles. To address this limitation, in this study, we propose a novel AMS based on online circulatory spectrophotometry (OCS) and incorporate debubbling, aeration, and segmented flow (DAS), named DAS-OCS-AMS. Initially, a debubbler is introduced to mitigate the issue of signal noise caused by bubbles (SNB). Subsequently, an aerated and segmented device is developed to address the issue of particle deposition on the inner wall of the pipeline (PDP) and on the windows of the flow cell (PDW). The proposed DAS-OCS-AMS is applied to monitor the kinetics of the photocatalytic degradation of Acid Orange Ⅱ by TiO2 (P25), and its results are compared with those obtained using the traditional OCS-AMS. The comparative analysis indicates that the proposed DAS-OCS-AMS effectively mitigates the influence of SNB, PDP, and PDW, yielding precise results both for the mixture and solid particles. The DAS-OCS-AMS provides a highly flexible universal framework for online circulatory automated monitoring and a robust hardware foundation for subsequent data processing research.
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<div class="JournalArticle Publication short-list"> <div class="authors"> <span class="author-name" > Chen, Y. </span> <span class="author-type"> </span> ; <span class="author-name" > Jiang, D. </span> <span class="author-type"> </span> ; <span class="author-name" > Zeng, C. </span> <span class="author-type"> </span> ; <span class="author-name" > Xu, C. </span> <span class="author-type"> </span> ; <span class="author-name" > Sun, H. </span> <span class="author-type"> </span> ; <span class="author-name" > Hou, Y. </span> <span class="author-type"> </span> ; <span class="author-name" > Zhou, M. ✉ </span> <span class="author-type"> </span> </div ><div class="title"><a href="/gui2/?mode=browse¶ms=publication;34750796" mtid="34750796" target="_blank">Controlling GaN-Based Laser Diode Performance by Variation of the Al Content of an Inserted AlGaN Electron Blocking Layer</a></div> <div class="pub-info"> <span class="journal-title">NANOMATERIALS</span> <span class="journal-volume">14</span> : <span class="journal-issue">5</span> <span class="page"> Paper: 449 </span> <span class="year">(2024)</span> </div> <div class="pub-end"><div class="identifier-list"> <span class="identifiers"> <span class="id identifier oa_none" title="none"> <a style="color:black" title="10.3390/nano14050449" target="_blank" href="https://doi.org/10.3390/nano14050449"> DOI </a> </span> <span class="id identifier oa_none" title="none"> <a style="color:black" title="001182900200001" target="_blank" href="https://www.webofscience.com/wos/woscc/full-record/001182900200001"> WoS </a> </span> <span class="id identifier oa_none" title="none"> <a style="color:black" title="85187476377" target="_blank" href="http://www.scopus.com/record/display.url?origin=inward&eid=2-s2.0-85187476377"> Scopus </a> </span> </span> </div> <div class="short-pub-prop-list"> <span class="short-pub-mtid"> Közlemény:34750796 </span> <span class="status-holder"><span class="status-data status-VALIDATED"> Egyeztetett </span></span> <span class="pub-core"> Idéző </span> <span class="pub-type">Folyóiratcikk (Szakcikk ) </span> <!-- && !record.category.scientific --> <span class="pub-category">Tudományos</span> </div> </div> </div><div class="JournalArticle Publication long-list"> <div class="authors"> <img title="Idézőközlemény" style="float: left" src="/frontend/resources/grid/publication-citation-icon.png"> <div class="autype autype0"> <span class="author-name" >Chen Y. </span> ; <span class="author-name" >Jiang D. </span> ; <span class="author-name" >Zeng C. </span> ; <span class="author-name" >Xu C. </span> ; <span class="author-name" >Sun H. </span> ; <span class="author-name" >Hou Y. </span> ; <span class="author-name" >Zhou M. ✉ </span> </div> </div> <div class="title"><a href="/gui2/?mode=browse¶ms=publication;34750796" target="_blank">Controlling GaN-Based Laser Diode Performance by Variation of the Al Content of an Inserted AlGaN Electron Blocking Layer</a></div> <div> <span class="journal-title">NANOMATERIALS</span> <span class="journal-issn">( <a target="_blank" href="https://portal.issn.org/resource/ISSN/2079-4991">2079-4991</a>)</span>: <span class="journal-volume">14</span> <span class="journal-issue">5</span> <span class="page"> Paper 449. </span> <span class="year">(2024)</span> </div> <div class="pub-footer"> <span class="language" xmlns="http://www.w3.org/1999/html">Nyelv: Angol | </span> <span class="identifiers"> <span class="id identifier oa_none" title="none"> <a style="color:black" title="10.3390/nano14050449" target="_blank" href="https://doi.org/10.3390/nano14050449"> DOI </a> </span> <span class="id identifier oa_none" title="none"> <a style="color:black" title="001182900200001" target="_blank" href="https://www.webofscience.com/wos/woscc/full-record/001182900200001"> WoS </a> </span> <span class="id identifier oa_none" title="none"> <a style="color:black" title="85187476377" target="_blank" href="http://www.scopus.com/record/display.url?origin=inward&eid=2-s2.0-85187476377"> Scopus </a> </span> </span> <div class="publication-citation"> <a target="_blank" href="/api/publication?cond=citations.related;eq;34750796&sort=publishedYear,desc&sort=title"> Idézett közlemények száma: 1 </a> </div> <div class="mtid"><span class="long-pub-mtid">Közlemény: 34750796</span> | <span class="status-data status-VALIDATED"> Egyeztetett </span> Idéző | <span class="type-subtype">Folyóiratcikk ( Szakcikk ) </span> | <span class="pub-category">Tudományos</span> | <span class="publication-sourceOfData">Scopus</span> </div> <div class="lastModified">Utolsó módosítás: 2024.03.21. 15:21 Bolgár Andrea (MFA admin 4) </div> </div></div>
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Developing prolonged antigen delivery systems that mimic long-term exposure to pathogens appears as a promising but still poorly explored approach to reach durable immunities. In this study, we have used a simple technology by which His-tagged proteins can be assembled, assisted by divalent cations, as supramolecular complexes with progressive complexity, namely protein-only nanoparticles and microparticles. Microparticles produced out of nanoparticles are biomimetics of secretory granules from the mammalian hormonal system. Upon subcutaneous administration, they slowly disintegrate, acting as an endocrine-like secretory system and rendering the building block nanoparticles progressively bioavailable. The performance of such materials, previously validated for drug delivery in oncology, has been tested here regarding the potential for time-prolonged antigen release. This has been completed by taking, as a building block, a nanostructured version of p30, a main structural immunogen from the African swine fever virus (ASFV). By challenging the system in both mice and pigs, we have observed unusually potent pro-inflammatory activity in porcine macrophages, and long-lasting humoral and cellular responses in vivo, which might overcome the need for an adjuvant. The robustness of both innate and adaptive responses tag, for the first time, these dynamic depot materials as a novel and valuable instrument with transversal applicability in immune stimulation and vaccinology.
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Correspondence Address: Kis, V.K.; HUN-REN Centre for Energy Research, Konkoly-Thege Miklós út 29-33, Hungary; email: kis.viktoria@ek.hun-ren.hu
Correspondence Address: Czigány, Z.; HUN-REN Centre for Energy Research, Konkoly-Thege Miklós út 29-33, Hungary; email: czigany.zsolt@ek.hun-ren.hu
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Multiphase nanomaterials are of increasing importance in material science. Providing reliable and statistically meaningful information on their average nanostructure is essential for synthesis control and applications. In this paper, we propose a novel procedure that simplifies and makes more effective the electron powder diffraction-based Rietveld analysis of nanomaterials. Our single step in-TEM method allows to obtain the instrumental broadening function of the TEM directly from a single measurement without the need for an additional X-ray diffraction measurement. Using a multilayer graphene calibration standard and applying properly controlled acquisition conditions on a spherical aberration-corrected microscope, we achieved the instrumental broadening of ±0.01 Å in terms of interplanar spacing. The shape of the diffraction peaks is modeled as a function of the scattering angle using the Caglioti relation, and the obtained parameters for instrumental broadening can be directly applied in the Rietveld analysis of electron diffraction data of the analyzed specimen. During peak shape analysis, the instrumental broadening parameters of the TEM are controlled separately from nanostructure-related peak broadening effects, which contribute to the higher reliability of nanostructure information extracted from electron diffraction patterns. The potential of the proposed procedure is demonstrated through the Rietveld analysis of hematite nanopowder and two-component Cu-Ni nanocrystalline thin film specimens.
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<div class="title"><a href="/gui2/?mode=browse¶ms=publication;34699351" target="_blank">Improved Method for Electron Powder Diffraction-Based Rietveld Analysis of Nanomaterials</a></div> <div> <span class="journal-title">NANOMATERIALS</span>
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<pre class="comment" style="margin-top: 0; margin-bottom: 0;"><u>Megjegyzés</u>: Export Date: 19 March 2024
Correspondence Address: Kis, V.K.; HUN-REN Centre for Energy Research, Konkoly-Thege Miklós út 29-33, Hungary; email: kis.viktoria@ek.hun-ren.hu
Correspondence Address: Czigány, Z.; HUN-REN Centre for Energy Research, Konkoly-Thege Miklós út 29-33, Hungary; email: czigany.zsolt@ek.hun-ren.hu</pre>
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Sub-nanometer-sized gold nanoclusters (Au NCs) were prepared via the spontaneous reduction of [AuCl4]−- ions with a hydroxamate derivative of L-tryptophan (Trp) natural amino acid (TrpHA). The prepared TrpHA-Au NCs possess intense blue emission (λem = 470 nm; λex = 380 nm) with a 2.13% absolute quantum yield and 1.47 ns average lifetime. The Trp-stabilized noble metal NCs are excellent metal ion sensors for Fe3+, but in this work, we highlighted that the incorporation of the hydroxamate functional group with an excellent metal ion binding capability can tune the selectivity and sensitivity of these NCs, which is a promising way to design novel strategies for the detection of other metal ions as well. Moreover, their simultaneous identification can also be realized. By decreasing the sensitivity of our nano-sensor for Fe3+ (limit of detection (LOD) ~11 µM), it was clearly demonstrated that the selectivity for Cu2+-ions can be significantly increased (LOD = 3.16 µM) in an acidic (pH = 3–4) condition. The surface-bounded TrpHA molecules can coordinate the Cu2+ confirmed by thermodynamic data, which strongly generates the linking of the NCs via the Cu2+ ions in acidic pH, and a parallel fluorescence quenching occurs. In the case of Fe3+, the degree of quenching strongly depends on the metal ion concentration, and it only occurs when the NCs are not able to bind more Fe3+ (~10 µM) on the surface, causing the NCs’ aggregation.
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<div class="JournalArticle Publication short-list"> <div class="authors"> <span class="author-name" > Vita, F. </span> <span class="author-type"> </span> ; <span class="author-name" > Adamo, F.C. </span> <span class="author-type"> </span> ; <span class="author-name" > Campana, M. </span> <span class="author-type"> </span> ; <span class="author-name" > Bordokas, B. </span> <span class="author-type"> </span> ; <span class="author-name" > Ciuchi, F. </span> <span class="author-type"> </span> ; <span class="author-name" > De, Santo M.P. </span> <span class="author-type"> </span> ; <span class="author-name" > Hermida-Merino, D. </span> <span class="author-type"> </span> ; <span class="author-name" > Lisovsky, A. </span> <span class="author-type"> </span> ; <span class="author-name" > Pisani, M. </span> <span class="author-type"> </span> ; <span class="author-name" > Pontoni, D. </span> <span class="author-type"> </span> et al. </div ><div class="title"><a href="/gui2/?mode=browse¶ms=publication;34745379" mtid="34745379" target="_blank">Macroscopic Biaxial Order in Multilayer Films of Bent-Core Liquid Crystals Deposited by Combined Langmuir–Blodgett/Langmuir–Schaefer Technique</a></div> <div class="pub-info"> <span class="journal-title">NANOMATERIALS</span> <span class="journal-volume">14</span> : <span class="journal-issue">4</span> <span class="page"> Paper: 357 </span> <span class="year">(2024)</span> </div> <div class="pub-end"><div class="identifier-list"> <span class="identifiers"> <span class="id identifier oa_none" title="none"> <a style="color:blue" title="10.3390/nano14040357" target="_blank" href="https://doi.org/10.3390/nano14040357"> DOI </a> </span> <span class="id identifier oa_none" title="none"> <a style="color:blue" title="001172477700001" target="_blank" href="https://www.webofscience.com/wos/woscc/full-record/001172477700001"> WoS </a> </span> <span class="id identifier oa_none" title="none"> <a style="color:blue" title="85185697183" target="_blank" href="http://www.scopus.com/record/display.url?origin=inward&eid=2-s2.0-85185697183"> Scopus </a> </span> </span> </div> <div class="short-pub-prop-list"> <span class="short-pub-mtid"> Közlemény:34745379 </span> <span class="status-holder"><span class="status-data status-VALIDATED"> Egyeztetett </span></span> <span class="pub-core"> Idéző </span> <span class="pub-type">Folyóiratcikk (Szakcikk ) </span> <!-- && !record.category.scientific --> <span class="pub-category">Tudományos</span> </div> </div> </div><div class="JournalArticle Publication long-list"> <div class="authors"> <img title="Idézőközlemény" style="float: left" src="/frontend/resources/grid/publication-citation-icon.png"> <div class="autype autype0"> <span class="author-name" >Vita F. </span> ; 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