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Anemophilous (wind‐driven) pollen is one type of primary biological aerosol particle, which can rupture under high humidity conditions and form smaller sub‐pollen particles (SPPs). Both pollen and SPPs can reach the upper troposphere under convective conditions, acting as cloud condensation nuclei (CCN) and ice nucleating particles (INPs), thus influencing cloud formation and precipitation. However, the impacts of these biological aerosols on cold cloud formation and local climate remain unclear as there are large uncertainties on their emission flux and ice nucleating abilities. Here, we incorporate pollen emission and rupture processes in the Weather Research and Forecasting Model with Chemistry (WRF‐Chem) simulations and update the Morrison microphysics scheme within WRF‐Chem using aerosol‐aware INP parameterizations to account for pollen in addition to other anthropogenic and biogenic aerosol. INP parameterizations for pollen and SPP are derived from laboratory experiments. When including pollen rupture rates as observed in a series of chamber studies, SPP concentrations increase, leading to an increase of cloud ice and water by up to 50% and potentially extending the duration of the convective system. Among all simulated hydrometeors, graupel and raindrops exhibit the largest enhancements from the inclusion of SPPs, with intensifying precipitation at the backside of the convective system and a greater spatial extent. Sensitivity simulations indicate that SPPs have a greater effect on cloud microphysical processes than whole pollen grains, and further observational evidence is needed to constrain these processes.
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<div class="JournalArticle Publication short-list"> <div class="authors"> <span class="author-name" > Zhang, Yingxiao </span> <span class="author-type"> </span> ; <span class="author-name" > Subba, Tamanna </span> <span class="author-type"> </span> ; <span class="author-name" > Matthews, Brianna H. </span> <span class="author-type"> </span> ; <span class="author-name" > Pettersen, Claire </span> <span class="author-type"> </span> ; <span class="author-name" > Brooks, Sarah D. </span> <span class="author-type"> </span> ; <span class="author-name" > Steiner, Allison L. </span> <span class="author-type"> </span> </div ><div class="title"><a href="/gui2/?mode=browse¶ms=publication;34734172" mtid="34734172" target="_blank">Effects of Pollen on Hydrometeors and Precipitation in a Convective System</a></div> <div class="pub-info"> <span class="journal-title">JOURNAL OF GEOPHYSICAL RESEARCH: ATMOSPHERES</span> <span class="journal-volume">129</span> : <span class="journal-issue">6</span> <span class="page"> pp. 1-24. , 24 p. </span> <span class="year">(2024)</span> </div> <div class="pub-end"><div class="identifier-list"> <span class="identifiers"> <span class="id identifier oa_none" title="none"> <a style="color:black" title="10.1029/2023JD039891" target="_blank" href="https://doi.org/10.1029/2023JD039891"> DOI </a> </span> <span class="id identifier oa_none" title="none"> <a style="color:black" title="https://agupubs.onlinelibrary.wiley.com/doi/10.1029/2023JD039891" target="_blank" href="https://agupubs.onlinelibrary.wiley.com/doi/10.1029/2023JD039891"> Egyéb URL </a> </span> </span> </div> <div class="short-pub-prop-list"> <span class="short-pub-mtid"> Közlemény:34734172 </span> <span class="status-holder"><span class="status-data status-APPROVED"> Nyilvános </span></span> <span class="pub-core"> Idéző </span> <span class="pub-type">Folyóiratcikk (Szakcikk ) </span> <!-- && !record.category.scientific --> <span class="pub-category">Tudományos</span> </div> </div> </div><div class="JournalArticle Publication long-list"> <div class="authors"> <img title="Idézőközlemény" style="float: left" src="/frontend/resources/grid/publication-citation-icon.png"> <div class="autype autype0"> <span class="author-name" >Zhang Yingxiao </span> ; <span class="author-name" >Subba Tamanna </span> ; <span class="author-name" >Matthews Brianna H. </span> ; <span class="author-name" >Pettersen Claire </span> ; <span class="author-name" >Brooks Sarah D. </span> ; <span class="author-name" >Steiner Allison L. </span> </div> </div> <div class="title"><a href="/gui2/?mode=browse¶ms=publication;34734172" target="_blank">Effects of Pollen on Hydrometeors and Precipitation in a Convective System</a></div> <div> <span class="journal-title">JOURNAL OF GEOPHYSICAL RESEARCH: ATMOSPHERES</span> <span class="journal-issn">(<a target="_blank" href="https://portal.issn.org/resource/ISSN/2169-897X">2169-897X</a> <a target="_blank" href="https://portal.issn.org/resource/ISSN/2169-8996">2169-8996</a>)</span>: <span class="journal-volume">129</span> <span class="journal-issue">6</span> <span class="page"> pp 1-24 </span> <span class="year">(2024)</span> </div> <div class="pub-footer"> <span class="language" xmlns="http://www.w3.org/1999/html">Nyelv: Angol | </span> <span class="identifiers"> <span class="id identifier oa_none" title="none"> <a style="color:black" title="10.1029/2023JD039891" target="_blank" href="https://doi.org/10.1029/2023JD039891"> DOI </a> </span> <span class="id identifier oa_none" title="none"> <a style="color:black" title="https://agupubs.onlinelibrary.wiley.com/doi/10.1029/2023JD039891" target="_blank" href="https://agupubs.onlinelibrary.wiley.com/doi/10.1029/2023JD039891"> Egyéb URL </a> </span> </span> <div class="publication-citation"> <a target="_blank" href="/api/publication?cond=citations.related;eq;34734172&sort=publishedYear,desc&sort=title"> Idézett közlemények száma: 1 </a> </div> <div class="mtid"><span class="long-pub-mtid">Közlemény: 34734172</span> | <span class="status-data status-APPROVED"> Nyilvános </span> Idéző | <span class="type-subtype">Folyóiratcikk ( Szakcikk ) </span> | <span class="pub-category">Tudományos</span> | <span class="publication-sourceOfData">kézi felvitel</span> </div> <div class="lastModified">Utolsó módosítás: 2024.03.12. 14:10 Makra László (Meteorológia) </div> </div></div>
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Correspondence Address: Szilagyi, J.; National Laboratory for Water Science and Water Security, Hungary; email: szilagyi.jozsef@emk.bme.hu
Funding details: Nemzeti Kutatási, Fejlesztési és Innovaciós Alap, NKFIA, RRF‐2.3.1‐21‐2022‐00008, TKP‐6‐6/PALY‐2021
Funding text 1: The author is grateful to Liming Wang for his readiness in answering questions and performing additional calculations, and for the reviewers whose comments led to important changes in the original text. Support provided by the (a) Ministry of Innovation and Technology of Hungary from the National Research, Development and Innovation Fund, financed under the TKP2021‐NVA (project# TKP‐6‐6/PALY‐2021), TKP2021‐BME‐NVA02 funding schemes and (b) Szechenyi Plan Plus program (project# RRF‐2.3.1‐21‐2022‐00008) is kindly acknowledged.
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Surprising significant underperformance of the polynomial complementary relationship (PCR) of evaporation (Szilagyi et al., 2017, https://doi.org/10.1002/2016jd025611) by Wang et al. (2023, https://doi.org/10.1029/2023jd038683) is caused by the (a) station-by-station application of a grid-based estimation procedure of the Priestley-Taylor parameter (α) value, and (b) choice of the wind function. Application of the Rome wind function in the Penman equation together with either a well-chosen single (constant) α or α as a function of the wet-environment air temperature, should result in much improved evaporation estimates by the PCR in line with previous studies. © 2024. American Geophysical Union. All Rights Reserved.
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<div class="JournalArticle Publication short-list"> <div class="authors"> <span class="author-name" mtid="10011332"> <a href="/gui2/?type=authors&mode=browse&sel=10011332" target="_blank">Szilagyi, Jozsef ✉</a> </span> <span class="author-type"> </span> </div ><div class="title"><a href="/gui2/?mode=browse¶ms=publication;34751434" mtid="34751434" target="_blank">Comment on “Comparison of the Efficiencies of the Prognostic Generalized Complementary Functions on Evaporation Estimation” by Wang, L., et al., Published in Journal of Geophysical Research: Atmospheres</a></div> <div class="pub-info"> <span class="journal-title">JOURNAL OF GEOPHYSICAL RESEARCH: ATMOSPHERES</span> <span class="journal-volume">129</span> : <span class="journal-issue">5</span> <span class="page"> Paper: 2023JD040070 , 4 p. </span> <span class="year">(2024)</span> </div> <div class="pub-end"><div class="identifier-list"> <span class="identifiers"> <span class="id identifier oa_none" title="none"> <a style="color:black" title="10.1029/2023JD040070" target="_blank" href="https://doi.org/10.1029/2023JD040070"> DOI </a> </span> <span class="id identifier oa_none" title="none"> <a style="color:black" title="85187171562" target="_blank" href="http://www.scopus.com/record/display.url?origin=inward&eid=2-s2.0-85187171562"> Scopus </a> </span> </span> </div> <div class="short-pub-prop-list"> <span class="short-pub-mtid"> Közlemény:34751434 </span> <span class="status-holder"><span class="status-data status-APPROVED"> Nyilvános </span></span> <span class="pub-core">Forrás </span> <span class="pub-type">Folyóiratcikk (Rövid közlemény ) </span> <!-- && !record.category.scientific --> <span class="pub-category">Tudományos</span> </div> </div> </div><div class="JournalArticle Publication long-list">
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<span class="authorAux-mtmt"> Hidrológia</span>)
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<div class="title"><a href="/gui2/?mode=browse¶ms=publication;34751434" target="_blank">Comment on “Comparison of the Efficiencies of the Prognostic Generalized Complementary Functions on Evaporation Estimation” by Wang, L., et al., Published in Journal of Geophysical Research: Atmospheres</a></div> <div> <span class="journal-title">JOURNAL OF GEOPHYSICAL RESEARCH: ATMOSPHERES</span>
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<div class="lastModified">Utolsó módosítás: 2024.03.22. 11:09 Andódy Katalin (BME admin4)
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<pre class="comment" style="margin-top: 0; margin-bottom: 0;"><u>Megjegyzés</u>: Export Date: 22 March 2024
Correspondence Address: Szilagyi, J.; National Laboratory for Water Science and Water Security, Hungary; email: szilagyi.jozsef@emk.bme.hu
Funding details: Nemzeti Kutatási, Fejlesztési és Innovaciós Alap, NKFIA, RRF‐2.3.1‐21‐2022‐00008, TKP‐6‐6/PALY‐2021
Funding text 1: The author is grateful to ...</pre>
</div></div>
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<div class="JournalArticle Publication short-list"> <div class="authors"> <span class="author-name" > Yu, Zeren </span> <span class="author-type"> </span> ; <span class="author-name" > Tian, Pengfei ✉ </span> <span class="author-type"> </span> ; <span class="author-name" > Kang, Chenliang </span> <span class="author-type"> </span> ; <span class="author-name" > Song, Xin </span> <span class="author-type"> </span> ; <span class="author-name" > Huang, Jianping </span> <span class="author-type"> </span> ; <span class="author-name" > Guo, Yumin </span> <span class="author-type"> </span> ; <span class="author-name" > Shi, Jinsen </span> <span class="author-type"> </span> ; <span class="author-name" > Tang, Chenguang </span> <span class="author-type"> </span> ; <span class="author-name" > Zhang, Haotian </span> <span class="author-type"> </span> ; <span class="author-name" > Zhang, Zhida </span> <span class="author-type"> </span> et al. </div ><div class="title"><a href="/gui2/?mode=browse¶ms=publication;34653145" mtid="34653145" target="_blank">Physical Properties, Chemical Components, and Transport Mechanisms of Atmospheric Aerosols Over a Remote Area on the South Slope of the Tibetan Plateau</a></div> <div class="pub-info"> <span class="journal-title">JOURNAL OF GEOPHYSICAL RESEARCH: ATMOSPHERES</span> <span class="journal-volume">129</span> : <span class="journal-issue">4</span> <span class="page"> Paper: e2023JD040193 , 19 p. </span> <span class="year">(2024)</span> </div> <div class="pub-end"><div class="identifier-list"> <span class="identifiers"> <span class="id identifier oa_none" title="none"> <a style="color:black" title="10.1029/2023JD040193" target="_blank" href="https://doi.org/10.1029/2023JD040193"> DOI </a> </span> <span class="id identifier oa_none" title="none"> <a style="color:blue" title="001158471800001" target="_blank" href="https://www.webofscience.com/wos/woscc/full-record/001158471800001"> WoS </a> </span> </span> </div> <div class="short-pub-prop-list"> <span class="short-pub-mtid"> Közlemény:34653145 </span> <span class="status-holder"><span class="status-data status-VALIDATED"> Egyeztetett </span></span> <span class="pub-core"> Idéző </span> <span class="pub-type">Folyóiratcikk (Szakcikk ) </span> <!-- && !record.category.scientific --> <span class="pub-category">Tudományos</span> </div> </div> </div><div class="JournalArticle Publication long-list">
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<div class="title"><a href="/gui2/?mode=browse¶ms=publication;34653145" target="_blank">Physical Properties, Chemical Components, and Transport Mechanisms of Atmospheric Aerosols Over a Remote Area on the South Slope of the Tibetan Plateau</a></div> <div> <span class="journal-title">JOURNAL OF GEOPHYSICAL RESEARCH: ATMOSPHERES</span>
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<div class="title"><a href="/gui2/?mode=browse¶ms=publication;34672809" target="_blank">One-Minute Resolution GOES-R Observations of Lamb and Gravity Waves Triggered by the Hunga Tonga-Hunga Ha'apai Eruptions on 15 January 2022</a></div> <div> <span class="journal-title">JOURNAL OF GEOPHYSICAL RESEARCH: ATMOSPHERES</span>
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<pre class="comment" style="margin-top: 0; margin-bottom: 0;"><u>Megjegyzés</u>: Meteorological Institute, Universität Hamburg, Hamburg, Germany
Northwest Research Associates, Boulder, CO, United States
Leibniz Institute of Atmospheric Physics, University of Rostock, Kühlungsborn, Germany
Export Date: 28 February 2024
Correspondence Address: Horváth, Á.; Meteorological Institute,...</pre>
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Due to limited direct measurements, regional or global terrestrial evapotranspiration (ET) is generally derived from a combination of meteorological and satellite observations. Although the inhomogeneity of the observed climate data has been widely reported, its impact on the calculated ET has not been adequately quantified. This study aimed to calculate ET using the modified Penman-Monteith (MPM) model with raw and homogenized meteorological data. Additionally, we compared the calculated ET with those estimates from variable methods (water balance, satellite-based, and reanalysis) in China and its six major river basins from 1982 to 2020. During the overlapping period of 1997-2018, ET calculated from raw input data decreased slightly at -0.39 mm yr(-2) (p = 0.64) in China, whereas homogenized ET showed a significant increasing trend of 0.93 mm yr(-2) (p = 0.02), with a better agreement with water balance ET (1.93 mm yr(-2), p = 0). Global Land Evaporation Amsterdam Model (GLEAM) and Modern-Era Retrospective Analysis for Research and Applications, version 2 (MERRA2) could reproduce the increasing trends with 2.08 mm yr(-2) (p = 0) and 2.59 mm yr(-2) (p = 0). The intercomparison of input variables (solar radiation, relative humidity, wind speed, precipitation, and air temperature) among ET products revealed substantial differences, which can account for the discrepancies in ET estimates. Homogenized ET, GLEAM and MERRA2 exhibited significant increasing trends in China and most river basins from 1982 to 2020. Our findings underscore the importance of utilizing homogenized input data for more accurate ET estimation.
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<div class="JournalArticle Publication short-list"> <div class="authors"> <span class="author-name" > Mao, Yuna </span> <span class="author-type"> </span> ; <span class="author-name" > Bai, Jiaxin </span> <span class="author-type"> </span> ; <span class="author-name" > Wu, Guocan </span> <span class="author-type"> </span> ; <span class="author-name" > Xu, Lin </span> <span class="author-type"> </span> ; <span class="author-name" > Yin, Changjian </span> <span class="author-type"> </span> ; <span class="author-name" > Feng, Fei </span> <span class="author-type"> </span> ; <span class="author-name" > He, Yanyi </span> <span class="author-type"> </span> ; <span class="author-name" > Zhang, Zhengtai </span> <span class="author-type"> </span> ; <span class="author-name" > Wang, Kaicun ✉ </span> <span class="author-type"> </span> </div ><div class="title"><a href="/gui2/?mode=browse¶ms=publication;34621111" mtid="34621111" target="_blank">Terrestrial Evapotranspiration Over China From 1982 to 2020: Consistency of Multiple Data Sets and Impact of Input Data</a></div> <div class="pub-info"> <span class="journal-title">JOURNAL OF GEOPHYSICAL RESEARCH: ATMOSPHERES</span> <span class="journal-volume">129</span> : <span class="journal-issue">3</span> <span class="page"> Paper: e2023JD039387 , 30 p. </span> <span class="year">(2024)</span> </div> <div class="pub-end"><div class="identifier-list"> <span class="identifiers"> <span class="id identifier oa_none" title="none"> <a style="color:blue" title="10.1029/2023JD039387" target="_blank" href="https://doi.org/10.1029/2023JD039387"> DOI </a> </span> <span class="id identifier oa_none" title="none"> <a style="color:blue" title="001158277700001" target="_blank" href="https://www.webofscience.com/wos/woscc/full-record/001158277700001"> WoS </a> </span> <span class="id identifier oa_none" title="none"> <a style="color:blue" title="85184407468" target="_blank" href="http://www.scopus.com/record/display.url?origin=inward&eid=2-s2.0-85184407468"> Scopus </a> </span> </span> </div> <div class="short-pub-prop-list"> <span class="short-pub-mtid"> Közlemény:34621111 </span> <span class="status-holder"><span class="status-data status-VALIDATED"> Egyeztetett </span></span> <span class="pub-core"> Idéző </span> <span class="pub-type">Folyóiratcikk (Szakcikk ) </span> <!-- && !record.category.scientific --> <span class="pub-category">Tudományos</span> </div> </div> </div><div class="JournalArticle Publication long-list">
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<div class="title"><a href="/gui2/?mode=browse¶ms=publication;34621111" target="_blank">Terrestrial Evapotranspiration Over China From 1982 to 2020: Consistency of Multiple Data Sets and Impact of Input Data</a></div> <div> <span class="journal-title">JOURNAL OF GEOPHYSICAL RESEARCH: ATMOSPHERES</span>
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Carbonate radical anion (CO3 center dot-) is generally overlooked in atmospheric chemistry. Our recent work emphasizes the important role of carbonate radicals produced on mineral dust surfaces in fast sulfate production under solar irradiation in the presence of CO2 at specifically low RH and light intensity. Yet so far how CO3 center dot- involves and affects secondary sulfate production under diverse RH, light intensity, and complex constituent matrix remains unknown, which essentially limits our comprehensive knowledge of CO(3)(center dot-)initiated SO2 oxidation scheme in the atmosphere. Herein, we explored the heterogeneous SO2 oxidation over both model and authentic dust and clays in the presence of CO2 at atmospheric relevant RHs and light intensities. Interestingly, we observe that CO2 promotes sulfate yield over authentic dust and clays at atmospheric-relevant RH and light intensity. This observation relates to the favorable kinetic between SO2 oxidation and CO3 center dot- while auto-quenching of these radical ions is largely minimized due to the sufficient sites of crustal constituents. Furthermore, employing a suite of authentic dust and machine learning strategies, we evaluated the relative importance of each constituent within airborne minerals or clays as well as environmental conditions including relative humidity, light intensity, and CO2 concentration in affecting SO2 uptake capability. On this basis, sulfate formation mediated by dust-driven pathway, accounting for nearly similar to 20.9% of overall contribution by the end of this century during some pollution episodes, even higher than gas-phase center dot OH (similar to 16.9%), will be increased by 163% if CO2-initiated SO2 oxidation scheme is incorporated. Plain Language Summary How carbonate radical ions involve and affect sulfate formation under different RHs, light intensities, and complex component matrices remains an open question. Secondary sulfate production is facilitated by CO3 center dot- over authentic dust particles in atmospheric relevant RH and light intensity. More importantly, this research emphasizes that CO2 is not an inert greenhouse gas that rarely participates in atmospheric chemistry but a strong oxidant precursor that will produce CO3 center dot- and subsequently trigger quick SO2 oxidation via chain reactions. This dust-driven reaction channel mediated by CO3 center dot- potentially contributes to nearly similar to 1/5 of secondary sulfate production during some pollution hours if the growing intensive anthropogenic activities continue.
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<div class="JournalArticle Publication short-list"> <div class="authors"> <span class="author-name" > Liu, Yangyang </span> <span class="author-type"> </span> ; <span class="author-name" > Wang, Tao </span> <span class="author-type"> </span> ; <span class="author-name" > Ge, Qiuyue </span> <span class="author-type"> </span> ; <span class="author-name" > You, Wenbo </span> <span class="author-type"> </span> ; <span class="author-name" > Li, Kejian </span> <span class="author-type"> </span> ; <span class="author-name" > Wang, Wei </span> <span class="author-type"> </span> ; <span class="author-name" > Xie, Lifang </span> <span class="author-type"> </span> ; <span class="author-name" > Wang, Longqian </span> <span class="author-type"> </span> ; <span class="author-name" > Fang, Xiaozhong </span> <span class="author-type"> </span> ; <span class="author-name" > Ruan, Xuejun </span> <span class="author-type"> </span> et al. </div ><div class="title"><a href="/gui2/?mode=browse¶ms=publication;34594292" mtid="34594292" target="_blank">Unveiling the Role of Carbonate Radical Anions in Dust-Driven SO<sub>2</sub> Oxidation</a></div> <div class="pub-info"> <span class="journal-title">JOURNAL OF GEOPHYSICAL RESEARCH: ATMOSPHERES</span> <span class="journal-volume">129</span> : <span class="journal-issue">3</span> <span class="page"> Paper: e2023JD040017 , 27 p. </span> <span class="year">(2024)</span> </div> <div class="pub-end"><div class="identifier-list"> <span class="identifiers"> <span class="id identifier oa_none" title="none"> <a style="color:black" title="10.1029/2023JD040017" target="_blank" href="https://doi.org/10.1029/2023JD040017"> DOI </a> </span> <span class="id identifier oa_none" title="none"> <a style="color:blue" title="001154957600001" target="_blank" href="https://www.webofscience.com/wos/woscc/full-record/001154957600001"> WoS </a> </span> <span class="id identifier oa_none" title="none"> <a style="color:black" title="85183923080" target="_blank" href="http://www.scopus.com/record/display.url?origin=inward&eid=2-s2.0-85183923080"> Scopus </a> </span> </span> </div> <div class="short-pub-prop-list"> <span class="short-pub-mtid"> Közlemény:34594292 </span> <span class="status-holder"><span class="status-data status-VALIDATED"> Egyeztetett </span></span> <span class="pub-core"> Idéző </span> <span class="pub-type">Folyóiratcikk (Szakcikk ) </span> <!-- && !record.category.scientific --> <span class="pub-category">Tudományos</span> </div> </div> </div><div class="JournalArticle Publication long-list">
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<img title="Idézőközlemény" style="float: left" src="/frontend/resources/grid/publication-citation-icon.png">
<div class="autype autype0"> <span class="author-name" >Liu Yangyang
</span>
;
<span class="author-name" >Wang Tao
</span>
;
<span class="author-name" >Ge Qiuyue
</span>
;
<span class="author-name" >You Wenbo
</span>
;
<span class="author-name" >Li Kejian
</span>
;
<span class="author-name" >Wang Wei
</span>
;
<span class="author-name" >Xie Lifang
</span>
;
<span class="author-name" >Wang Longqian
</span>
;
<span class="author-name" >Fang Xiaozhong
</span>
;
<span class="author-name" >Ruan Xuejun
</span>
;
<span class="author-name" >Yang Le
</span>
;
<span class="author-name" >Wang Runbo
</span>
;
<span class="author-name" >Zhang Liwu ✉
</span>
</div>
</div>
<div class="title"><a href="/gui2/?mode=browse¶ms=publication;34594292" target="_blank">Unveiling the Role of Carbonate Radical Anions in Dust-Driven SO<sub>2</sub> Oxidation</a></div> <div> <span class="journal-title">JOURNAL OF GEOPHYSICAL RESEARCH: ATMOSPHERES</span>
<span class="journal-issn">(<a target="_blank" href="https://portal.issn.org/resource/ISSN/2169-897X">2169-897X</a> <a target="_blank" href="https://portal.issn.org/resource/ISSN/2169-8996">2169-8996</a>)</span>:
<span class="journal-volume">129</span> <span class="journal-issue">3</span>
<span class="page">
Paper e2023JD040017.
27 p.
</span> <span class="year">(2024)</span>
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Humic-like substances (HULIS) are a ubiquitous reactive component of atmospheric aerosol. They participate in the formation of secondary organic aerosols via chemical reactions with atmospheric oxidants. Here, we assess the influence of transition metal ions (namely ferric iron, Fe(III)), and nitrate ions (NO3-) on the heterogeneous reaction of gaseous NO2 with an aqueous film containing gallic acid (GA) or tannic acid (TA) as proxies for HULIS. Using a vertical wetted wall flow tube technique, the uptake coefficients of gaseous NO2 on GA and TA increased nonlinearly with increasing [Fe(III)], in dark and under light irradiation. However, the combined effect of both ions, Fe(III) and NO3-, led to a substantial decrease in NO2 uptake in the dark and under simulated near-UV sunlight irradiation (300 < lambda < 400 nm). The lifetime of GA in dilute aqueous phase, which corresponds to cloud water, due to reaction with NO2 would be 6 hr during both nighttime and daytime. However, the lifetime of GA in aerosol particles which contain both ions, that is, Fe(III) and NO3-, would increase to 27 hr during nighttime and 11 days and 6 hr due to light-induced reaction with NO2. Also, we observed, using Fourier transform ion cyclotron resonance mass spectrometry, the formation of nitrocatechols compounds (e.g., methyl-nitrocatechol), which contribute to brown carbon. Compounds with reduced functional groups such as amines were also observed in the presence of iron and nitrate ions in the dark and under irradiation, indicating that Fe(III) and NO3-, can influence the kinetics and product distribution in deliquescent aerosol particles.
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<div class="JournalArticle Publication short-list"> <div class="authors"> <span class="author-name" > Li, Pan </span> <span class="author-type"> </span> ; <span class="author-name" > Mekic, Majda </span> <span class="author-type"> </span> ; <span class="author-name" > Wang, Yiqun </span> <span class="author-type"> </span> ; <span class="author-name" > He, Bowen </span> <span class="author-type"> </span> ; <span class="author-name" > Deng, Huifan </span> <span class="author-type"> </span> ; <span class="author-name" > Xu, Jinli </span> <span class="author-type"> </span> ; <span class="author-name" > Pang, Hongwei </span> <span class="author-type"> </span> ; <span class="author-name" > Jiang, Bin </span> <span class="author-type"> </span> ; <span class="author-name" > Tang, Mingjin </span> <span class="author-type"> </span> ; <span class="author-name" > Wang, Xinming </span> <span class="author-type"> </span> et al. </div ><div class="title"><a href="/gui2/?mode=browse¶ms=publication;34578493" mtid="34578493" target="_blank">Impact of Nitrate and Iron Ions on Uptake Coefficients and Condensed Phase Products From the Reaction of Gaseous NO<sub>2</sub> With HULIS Proxies</a></div> <div class="pub-info"> <span class="journal-title">JOURNAL OF GEOPHYSICAL RESEARCH: ATMOSPHERES</span> <span class="journal-volume">129</span> : <span class="journal-issue">3</span> <span class="page"> Paper: e2023JD039698 , 17 p. </span> <span class="year">(2024)</span> </div> <div class="pub-end"><div class="identifier-list"> <span class="identifiers"> <span class="id identifier oa_none" title="none"> <a style="color:blue" title="10.1029/2023JD039698" target="_blank" href="https://doi.org/10.1029/2023JD039698"> DOI </a> </span> <span class="id identifier oa_none" title="none"> <a style="color:blue" title="001156391400001" target="_blank" href="https://www.webofscience.com/wos/woscc/full-record/001156391400001"> WoS </a> </span> <span class="id identifier oa_none" title="none"> <a style="color:blue" title="85184197793" target="_blank" href="http://www.scopus.com/record/display.url?origin=inward&eid=2-s2.0-85184197793"> Scopus </a> </span> </span> </div> <div class="short-pub-prop-list"> <span class="short-pub-mtid"> Közlemény:34578493 </span> <span class="status-holder"><span class="status-data status-VALIDATED"> Egyeztetett </span></span> <span class="pub-core"> Idéző </span> <span class="pub-type">Folyóiratcikk (Szakcikk ) </span> <!-- && !record.category.scientific --> <span class="pub-category">Tudományos</span> </div> </div> </div><div class="JournalArticle Publication long-list">
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<div class="autype autype0"> <span class="author-name" >Li Pan
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;
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;
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;
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;
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;
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;
<span class="author-name" >Gligorovski Sasho ✉
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<div class="title"><a href="/gui2/?mode=browse¶ms=publication;34578493" target="_blank">Impact of Nitrate and Iron Ions on Uptake Coefficients and Condensed Phase Products From the Reaction of Gaseous NO<sub>2</sub> With HULIS Proxies</a></div> <div> <span class="journal-title">JOURNAL OF GEOPHYSICAL RESEARCH: ATMOSPHERES</span>
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<span class="journal-volume">129</span> <span class="journal-issue">3</span>
<span class="page">
Paper e2023JD039698.
17 p.
</span> <span class="year">(2024)</span>
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