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The microwave spectra of the parent and one deuterated species (hydroxyl group) have been investigated in the 26.5 39.5 GHz spectral region at - 15-degrees-C. One conformer was assigned. This rotamer is stabilized by an intramolecular hydrogen bond formed between the hydrogen atom of the hydroxyl group and the pseudo-pi electrons on the outside of the nearest C-C edge of the cyclopropyl ring. The identified conformer is shown to be present in a concentration of 10-30% of the total. The electron diffraction data are in accordance with the presence of three 2-cyclopropylethanol conformers, each being characterized by the dihedral angles associated with the C2-C3, C1-C2 and C1-O1 bonds, as follows: G + /G + /G-(48.6 %); G + /G -/A (19.7 %); G + /A/A (31.7 %). The most abundant conformer is the one that was identified from the microwave spectrum. 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