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"publishedYear" : 2006, "abstractText" : "Nowadays, time-resolved spectroscopy data can be routinely and accurately collected in UV–vis femtosecond transient absorption spectroscopy. However, the data analysis strategy and the postulation of a physically valid model for this kind of measurements may be tackled with many different approaches ranging from pure soft-modeling (model-free) to hard-modeling, where the elaboration of a parametric spectro-temporal model may be required. This paper reviews methods that are used in practice for the analysis of femtosecond transient absorption spectroscopy data. Model-based methods, common in photochemistry, are revisited, and soft-modeling methods, which originate from the chemometrics field and that recently disseminated in the photo(bio)chemistry literature, are presented. These soft-modeling methods are designed to suit the intrinsic nature of the multivariate (or multi-way) measurement. Soft-modeling tools do not require a priori physical or mechanistic models to provide a decomposition of the data on the time and wavelength dimensions, the only requirement being that these two (or more) dimensions are separable. Additionally, Bayesian data analysis, which provides a probabilistic framework for data analysis, is considered in detail, since it allows uncertainty quantification and validation of the model selection step.", "subjects" : [ { "otype" : "Classification", "mtid" : 10154, "link" : "/api/classification/10154", "label" : "Fizika", "published" : true, "snippet" : true } ], "digital" : null, "printed" : null, "sourceYear" : 2010, "packet" : "209112", "foreignEdition" : true, "foreignLanguage" : true, "fullPublication" : true, "conferencePublication" : false, "nationalOrigin" : null, "missingAuthor" : false, "oaType" : "NONE", "oaCheckDate" : "2024-02-13", "oaFree" : false, "citationCount" : 14, "citationCountUnpublished" : 0, "citationCountWoOther" : 14, "independentCitCountWoOther" : 11, "nationalOriginCitationCount" : 2, "foreignEditionCitationCount" : 13, "doiCitationCount" : 12, "wosCitationCount" : 12, "scopusCitationCount" : 13, "wosScopusCitationCount" : 13, 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