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"Journal", "mtid" : 1315, "link" : "/api/journal/1315", "label" : "DIAMOND AND RELATED MATERIALS 0925-9635 1879-0062", "pIssn" : "0925-9635", "eIssn" : "1879-0062", "reviewType" : "REVIEWED", "noIF" : false, "sciIndexed" : true, "scopusIndexed" : true, "lang" : "FOREIGN", "hungarian" : false, "published" : true, "oldId" : 1315, "snippet" : true }, "volume" : "14", "issue" : "3-7", "firstPage" : "1041", "lastPage" : "1046", "firstPageOrInternalIdForSort" : "1041", "pageLength" : 6, "publishedYear" : 2005, "abstractText" : "A well defined structure in the photoluminescence excitation (PLE) spectrum of several hydrogenated amorphous carbon (a-C:H) films have been observed. An intense band appears in the PLE spectrum at excitation photon energies below optical gap and the other band of a much weaker intensity compared to the low energy peak can be observed for excitations in the vicinity of band-to-band optical transitions. The low energy band of the PLE spectrum exhibits resonance features and its peak position is in a close relation with the energy of the photoluminescence (PL) band maximum; that is when the PLE maximum corresponding to the blue PL band is shifted to higher photon energy relatively to that of the green PL band. In contrast to this behavior the high energy band maximum of PLE appears, practically at the same photon energy for both the green and the blue bands measured in the same a-C:H sample. In the framework of the luminescence mechanism for a-C:H the observed characteristic features of PLE spectra is explained by optical excitation inside the luminescence centers, at which spatial confinement of the electron hole pairs takes place and by optical transitions in the neighborhood of the luminescence centers to a some extended states as well. © 2005 Elsevier B.V. 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